ICCAS OpenIR
Synthesis of Bisflavanol-Type Natural Products and Their Analogues- via Self-Coupling of C8-Methylol Catechin Derivatives
Huang, Deng-Ming; Li, Hui-Jing; Zhao, Yan; Wu, Yan-Chao l
2019-08-16
Source PublicationSYNTHESIS-STUTTGART
ISSN0039-7881
Volume51Issue:16Pages:3127-3141
AbstractA highly efficient and regioselective self-coupling of C8-methylol catechin derivatives is developed for the synthesis of dimeric flavanol analogues under metal-free and mild conditions. Its applicability is showcased by the efficient synthesis of bisflavanol-type natural products bis-8,8 '-catechinylmethane, bis-8,8 '-epicatechinylmethane, talienbisflavan A, and oolonghomobisflavan A. The novel self-coupling mechanism sheds new light on the classical Friedel-Crafts alkylation mechanism in acid-catalyzed catechin-formaldehyde condensation.
DOI10.1055/s-0037-1610707
Indexed BySCI
Language英语
WOS IDWOS:000477973200010
EI Accession Number1437-210X
Citation statistics
Document Type期刊论文
Identifierhttp://ir.iccas.ac.cn/handle/121111/82656
Collection中国科学院化学研究所
AffiliationChinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Huang, Deng-Ming,Li, Hui-Jing,Zhao, Yan,et al. Synthesis of Bisflavanol-Type Natural Products and Their Analogues- via Self-Coupling of C8-Methylol Catechin Derivatives[J]. SYNTHESIS-STUTTGART,2019,51(16):3127-3141.
APA Huang, Deng-Ming,Li, Hui-Jing,Zhao, Yan,&Wu, Yan-Chao l.(2019).Synthesis of Bisflavanol-Type Natural Products and Their Analogues- via Self-Coupling of C8-Methylol Catechin Derivatives.SYNTHESIS-STUTTGART,51(16),3127-3141.
MLA Huang, Deng-Ming,et al."Synthesis of Bisflavanol-Type Natural Products and Their Analogues- via Self-Coupling of C8-Methylol Catechin Derivatives".SYNTHESIS-STUTTGART 51.16(2019):3127-3141.
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