ICCAS OpenIR
A simplified formulation of linear and nonlinear spectroscopy of ordered molecular systems
Wang, HF
2004-06-01
Source PublicationCHINESE JOURNAL OF CHEMICAL PHYSICS
ISSN1003-7713
Volume17Issue:3Pages:362-368
AbstractA simplified formulation for treating the linear and nonlinear spectroscopy of ordered molecular systems is presented, in order to help experimentalists to have an explicit physical picture and quantitative tool on using linear and nonlinear spectroscopy to study molecules in ordered molecular systems. This formulation is expended from our recent quantitative orientational and polarization treatment on second-order nonlinear spectroscopic techniques in interface studies, namely, the Second Harmonic Generation (SHG) and Sum Frequency Generation-Vibrational Polarization Spectroscopy (SFG-VPS). The key to this formulation is to simplify the effective linear or nonlinear molecular susceptibility and construct the general orientational functional with a clear approach to calculate the orientational and intensity parameters from the experimental parameters, which deter-mines the orientational and polarization behavior of the general orientational functional in a particular experimental configuration. Also discussed are the advantages of coherent spectroscopic techniques over incoherent ones for the accurate measurement of orientation and ordering of ordered molecular system.
KeywordLinear And nonLinear Spectroscopy Second Harmonic Generation Sum Frequency Generation Vibrational Spectroscopy General Orientational Functional Ordered Molecular System
Indexed BySCI
Language英语
WOS IDWOS:000222521100022
PublisherSCIENCE CHINA PRESS
Citation statistics
Cited Times:21[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.iccas.ac.cn/handle/121111/81564
Collection中国科学院化学研究所
Corresponding AuthorWang, HF
AffiliationChinese Acad Sci, Inst Chem, Ctr Mol Sci, State Key Lab Mol React Dynam, Beijing 100080, Peoples R China
Recommended Citation
GB/T 7714
Wang, HF. A simplified formulation of linear and nonlinear spectroscopy of ordered molecular systems[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2004,17(3):362-368.
APA Wang, HF.(2004).A simplified formulation of linear and nonlinear spectroscopy of ordered molecular systems.CHINESE JOURNAL OF CHEMICAL PHYSICS,17(3),362-368.
MLA Wang, HF."A simplified formulation of linear and nonlinear spectroscopy of ordered molecular systems".CHINESE JOURNAL OF CHEMICAL PHYSICS 17.3(2004):362-368.
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