ICCAS OpenIR
Linear and Cyclic Tetrathiafulvalene-Naphthalenediimide Donor-Acceptor Molecules: Metal Ions-Promoted Electron Transfer
Tan, Luxi1,2; Zhang, Guanxin1; Zhang, Deqing1; Zhu, Daoben1
2011-11-04
Source PublicationJOURNAL OF ORGANIC CHEMISTRY
ISSN0022-3263
Volume76Issue:21Pages:9046-9052
AbstractThree linear and one cyclic tetrathiafulvalene-1,4,5,8-naphthalenediimide (TTF-NDI) compounds 1, 2, 3, and 4 were synthesized and studied in the presence of metal ions. Both absorption and electron spin resonance spectroscopic studies clearly indicate that electron transfer occurs from TTF to the NDI unit in the presence of metal ions (Pb2+ and Sc3+) for linear compounds 1 and 2. The mechanism based on the metal ion coordination is proposed for the electron transfer within 1 and 2 after the addition of metal ions. Compound 3 exhibits intramolecular charge-transfer absorption because of the cydophane framework. Interestingly, intramolecular electron transfer also takes place for 3 after the addition of either Sc3+ or Pb2+.
DOI10.1021/jo201802p
Indexed BySCI ; IC
Language英语
WOS IDWOS:000296206400045
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:16[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.iccas.ac.cn/handle/121111/73712
Collection中国科学院化学研究所
Corresponding AuthorZhang, Deqing
Affiliation1.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Organ Solids Lab, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Tan, Luxi,Zhang, Guanxin,Zhang, Deqing,et al. Linear and Cyclic Tetrathiafulvalene-Naphthalenediimide Donor-Acceptor Molecules: Metal Ions-Promoted Electron Transfer[J]. JOURNAL OF ORGANIC CHEMISTRY,2011,76(21):9046-9052.
APA Tan, Luxi,Zhang, Guanxin,Zhang, Deqing,&Zhu, Daoben.(2011).Linear and Cyclic Tetrathiafulvalene-Naphthalenediimide Donor-Acceptor Molecules: Metal Ions-Promoted Electron Transfer.JOURNAL OF ORGANIC CHEMISTRY,76(21),9046-9052.
MLA Tan, Luxi,et al."Linear and Cyclic Tetrathiafulvalene-Naphthalenediimide Donor-Acceptor Molecules: Metal Ions-Promoted Electron Transfer".JOURNAL OF ORGANIC CHEMISTRY 76.21(2011):9046-9052.
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