ICCAS OpenIR
Double Ionization of Nitrogen from Multiple Orbitals
Wu, Zhifeng1; Wu, Chengyin1; Liu, Xianrong1; Deng, Yongkai1; Gong, Qihuang1; Song, Di2; Su, Hongmei2
2010-07-01
Source PublicationJOURNAL OF PHYSICAL CHEMISTRY A
ISSN1089-5639
Volume114Issue:25Pages:6751-6756
AbstractIn intense femtosecond laser fields, molecules could be tunnel ionized from multiple valence orbitals, which produces molecular ions in different electronic states. In this article, we have used a reaction microscope to study double ionization of nitrogen by intense femtosecond laser pulses. It is found that some doubly charged molecular ions N(2)(2+) are metastable while others dissociate through charge symmetric dissociation (N(2)(2+) -> N(+) + N(+)) or charge asymmetric dissociation (N(2)(2+) -> N(2+) + N). The kinetic energy releases and angular distributions of atomic ions are measured for the dissociation channels. With the aid of the CASSCF and MRCI calculations, the electronic states are identified and the contributions of the valence orbitals are discussed for these dissociated molecular dications.
DOI10.1021/jp1018197
Indexed BySCI
Language英语
WOS IDWOS:000278981900003
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:24[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.iccas.ac.cn/handle/121111/70832
Collection中国科学院化学研究所
Corresponding AuthorWu, Chengyin
Affiliation1.Peking Univ, Dept Phys, State Key Lab Mesoscop Phys, Beijing 100871, Peoples R China
2.Chinese Acad Sci, Inst Chem, BNLMS, State Key Lab Mol React Dynam, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Wu, Zhifeng,Wu, Chengyin,Liu, Xianrong,et al. Double Ionization of Nitrogen from Multiple Orbitals[J]. JOURNAL OF PHYSICAL CHEMISTRY A,2010,114(25):6751-6756.
APA Wu, Zhifeng.,Wu, Chengyin.,Liu, Xianrong.,Deng, Yongkai.,Gong, Qihuang.,...&Su, Hongmei.(2010).Double Ionization of Nitrogen from Multiple Orbitals.JOURNAL OF PHYSICAL CHEMISTRY A,114(25),6751-6756.
MLA Wu, Zhifeng,et al."Double Ionization of Nitrogen from Multiple Orbitals".JOURNAL OF PHYSICAL CHEMISTRY A 114.25(2010):6751-6756.
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