ICCAS OpenIR
Rational Design of Low-Temperature Hydrogenation Catalysts: Theoretical Predictions and Experimental Verification
Chen, Jingguang G.1; Qi Sui-Tao1,2; Humbert, Michael P.1; Menning, Carl A.1; Zhu Yue-Xiang3
2010-04-01
Source PublicationACTA PHYSICO-CHIMICA SINICA
ISSN1000-6818
Volume26Issue:4Pages:869-876
AbstractIn this review, we will provide a brief review of our recent theoretical and experimental studies of bimetallic surfaces and catalysts for the low-temperature hydrogenation of unsaturated C=C and C=O bonds. We will first use the hydrogenation of cyclohexene as a probe reaction to demonstrate the importance of using several parallel approaches. including fundamental surface science and density functional theory (DFT) studies on single crystal surfaces, synthesis. and characterization of polycrystalline surfaces and supported catalysts, and reactor evaluation of supported catalysts. We will then provide a summary of applications of bimetallic catalysts for other hydrogenation reactions, including the selective hydrogenation of the C=O bond in acrolein. the low-temperature hydrogenation of benzene. and the selective hydrogenation of acetylene in the presence of ethylene Finally, we will discuss the possibility of replacing the platinum (Pt) component with metal carbides to reduce the loading of Pt in bimetallic catalysts
KeywordHydrogenation Bimetallic Catalyst Metal Carbide Density Functional Calculation
DOI10.3866/PKU.WHXB20100441
Indexed BySCI
Language英语
WOS IDWOS:000276958400012
PublisherPEKING UNIV PRESS
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Cited Times:19[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.iccas.ac.cn/handle/121111/69410
Collection中国科学院化学研究所
Corresponding AuthorChen, Jingguang G.
Affiliation1.Univ Delaware, Ctr Catalyt Sci & Technol, Dept Chem Engn, Newark, DE 19716 USA
2.Xi An Jiao Tong Univ, Dept Chem Engn, Xian 710049, Peoples R China
3.Peking Univ, Coll Chem & Mol Engn, State Key Lab Struct Chem Unstable & Stable Speci, Beijing Natl Lab Mol Sci, Beijing 100871, Peoples R China
Recommended Citation
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Chen, Jingguang G.,Qi Sui-Tao,Humbert, Michael P.,et al. Rational Design of Low-Temperature Hydrogenation Catalysts: Theoretical Predictions and Experimental Verification[J]. ACTA PHYSICO-CHIMICA SINICA,2010,26(4):869-876.
APA Chen, Jingguang G.,Qi Sui-Tao,Humbert, Michael P.,Menning, Carl A.,&Zhu Yue-Xiang.(2010).Rational Design of Low-Temperature Hydrogenation Catalysts: Theoretical Predictions and Experimental Verification.ACTA PHYSICO-CHIMICA SINICA,26(4),869-876.
MLA Chen, Jingguang G.,et al."Rational Design of Low-Temperature Hydrogenation Catalysts: Theoretical Predictions and Experimental Verification".ACTA PHYSICO-CHIMICA SINICA 26.4(2010):869-876.
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