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Catalytic CO Oxidation by O-2 Mediated by Noble-Metal-Free Cluster Anions Cu2VO3-5-
Wang, Li-Na; Li, Xiao-Na; Jiang, Li-Xue; Yang, Bin; Liu, Qing-Yu; Xu, Hong-Guang; Zheng, Wei-Jun; He, Sheng-Gui
MAR 19 2018
Source PublicationANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume57Issue:13Pages:3349-3353
AbstractCatalytic CO oxidation by molecular O-2 is an important model reaction in both the condensed phase and gas-phase studies. Available gas-phase studies indicate that noble metal is indispensable in catalytic CO oxidation by O-2 under thermal collision conditions. Herein, we identified the first example of noble-metal-free heteronuclear oxide cluster catalysts, the copper-vanadium bimetallic oxide clusters Cu2VO3-5- for CO oxidation by O-2. The reactions were characterized by mass spectrometry, photoelectron spectroscopy, and density functional calculations. The dynamic nature of the Cu-Cu unit in terms of the electron storage and release is the driving force to promote CO oxidation and O-2 activation during the catalysis.
Document Type期刊论文
Identifierhttp://ir.iccas.ac.cn/handle/121111/38707
Collection其它
Recommended Citation
GB/T 7714
Wang, Li-Na,Li, Xiao-Na,Jiang, Li-Xue,et al. Catalytic CO Oxidation by O-2 Mediated by Noble-Metal-Free Cluster Anions Cu2VO3-5-[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,MAR ,57(13):3349-3353.
APA Wang, Li-Na.,Li, Xiao-Na.,Jiang, Li-Xue.,Yang, Bin.,Liu, Qing-Yu.,...&He, Sheng-Gui.(MAR ).Catalytic CO Oxidation by O-2 Mediated by Noble-Metal-Free Cluster Anions Cu2VO3-5-.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,57(13),3349-3353.
MLA Wang, Li-Na,et al."Catalytic CO Oxidation by O-2 Mediated by Noble-Metal-Free Cluster Anions Cu2VO3-5-".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 57.13(MAR ):3349-3353.
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