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题名: Efficient hydrogenolysis of 5-hydroxymethylfurfural to 2,5-dimethylfuran over a cobalt and copper bimetallic catalyst on N-graphene-modified Al2O3
作者: Guo, Weiwei1, 2; Liu, Hangyu1, 2; Zhang, Suqi1; Han, Hongling1, 2; Liu, Huizhen1, 2; Jiang, Tao1; Han, Buxing1, 2; Wu, Tianbin1
刊名: GREEN CHEMISTRY
发表日期: 2016
卷: 18, 期:23, 页:6222-6228
收录类别: SCI
英文摘要: 2,5-Dimethylfuran (DMF) is an important candidate for liquid fuels and can be produced from biomass derived 5-hydroxymethylfurfural (HMF). Efficient transformation of HMF to DMF has not been achieved over a non-noble catalyst under milder conditions. Herein, we developed a copper and cobalt bimetallic nanoparticle catalyst supported on N-graphene-modified Al2O3 (CuCo (R)/NGr/alpha-Al2O3). It was found that CuCo (R)/NGr/alpha-Al2O3 could catalyze the conversion of HMF to DMF effectively and the yield of DMF could reach 99%. The catalyst was completely not active for the hydrogenation of the CvC bond in furan and thus no 2,5-bis (hydroxymethyl) tetrahydrofuran (DHTHF) and 2,5-dimethyltetrahydrofuran (DMTHF) were detected.
语种: 英语
内容类型: 期刊论文
URI标识: http://ir.iccas.ac.cn/handle/121111/36518
Appears in Collections:胶体、界面与化学热力学实验室_期刊论文

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作者单位: 1.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, CAS Key Lab Colloid & Interface & Thermodynam, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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