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ICCAS OpenIR  > 分子纳米结构与纳米技术实验室  > 期刊论文
题名: Nitrogen, Phosphorus, and Sulfur Co-Doped Hollow Carbon Shell as Superior Metal-Free Catalyst for Selective Oxidation of Aromatic Alkanes
作者: Yang, Shuliang1; Peng, Li2; Huang, Peipei1; Wang, Xiaoshi1; Sun, Yongbin1; Cao, Changyan1; Song, Weiguo1
关键词: carbon ; doping ; heterogeneous catalysis ; metal-free catalysts ; selective oxidation
刊名: ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
发表日期: 2016-03-14
卷: 55, 期:12, 页:4016-4020
收录类别: SCI ; CCR
英文摘要: Metal-free heteroatom-doped carbocatalysts with a high surface area are desirable for catalytic reactions. In this study, we found an efficient strategy to prepare nitrogen, phosphorus, and sulfur co-doped hollow carbon shells (denote as NPS-HCS) with a surface area of 1020m(2)g(-1). Using a poly(cyclotriphosphazene-co-4,4-sulfonyldiphenol) (PZS) shell as carbon source and N, P, S-doping source, and the ZIF-67 core as structural template as well as extra N-doping source, NPS-HCS were obtained with a high surface area and superhydrophilicity. All these features render the prepared NPS-HCS a superior metal-free carbocatalyst for the selective oxidation of aromatic alkanes in aqueous solution. This study provides a reliable and facile route to prepare doped carbocatalysts with enhanced catalytic properties.
语种: 英语
内容类型: 期刊论文
URI标识: http://ir.iccas.ac.cn/handle/121111/35959
Appears in Collections:分子纳米结构与纳米技术实验室_期刊论文

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作者单位: 1.Chinese Acad Sci, Inst Chem, Lab Mol Nanostruct & Nanotechnol, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China
2.EPFL, EPFL ISIC Valais, Inst Chem Sci & Engn, CH-1950 Sion, Switzerland
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