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题名: Organocatalytic Enantioselective Reaction of Cyclopent-2-enone-Derived Morita-Baylis-Hillman Alcohols with 4-Hydroxycoumarins
作者: Ren, Chuanli1, 2; Wei, Feng1; Xuan, Qingqing1; Wang, Dong1; Liu, Li1
关键词: Bronsted acids ; chiral primary amines ; iminium catalysis ; pyranocoumarins ; tandem reactions
刊名: ADVANCED SYNTHESIS & CATALYSIS
发表日期: 2016-01-07
卷: 358, 期:1, 页:132-137
收录类别: SCI
英文摘要: A direct enantioselective reaction of cyclopent-2-enone-derived Morita-Baylis-Hillman alcohols with 4-hydroxycoumarins has been developed under the catalysis of a chiral primary amine derived from cinchonine in combination with a Bronsted acid. The reaction provides pyranocoumarin products with three vicinal chiral carbon centers in highly regio-, diastereo- and enantioselectivities through a tandem allylic alkylation/intramolecular oxa-Michael addition.
语种: 英语
内容类型: 期刊论文
URI标识: http://ir.iccas.ac.cn/handle/121111/35825
Appears in Collections:分子识别与功能实验室_期刊论文

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作者单位: 1.Chinese Acad Sci, Inst Chem, CAS Key Lab Mol Recognit & Funct, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China
2.Qingdao Univ Sci & Technol, Sch Polymer Sci & Engn, Qingdao 266042, Peoples R China
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