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题名: Effect of Pulse Shaping on Observing Coherent Energy Transfer in Single Light-Harvesting Complexes
作者: Song, Kai1; Bai, Shuming1, 2; Shi, Qiang1, 2
刊名: JOURNAL OF PHYSICAL CHEMISTRY B
发表日期: 2016-11-17
卷: 120, 期:45, 页:11637-11643
收录类别: SCI
英文摘要: Recent experimental and theoretical studies have revealed that quantum coherence plays an important role in the excitation energy transfer in photosynthetic light harvesting (LH) complexes. Inspired by the recent single-molecule two-color double-pump experiment, we theoretically investigate the effect of pulse shaping on observing coherent energy transfer in the single bacterial LH2 complex. It is found that quantum coherent energy transfer can be observed when the time delay and phase difference between the two laser pulses are controlled independently. However, when the two-color pulses are generated using the pulse-shaping method, how the laser pulses are prepared is crucial to the observation of quantum coherent energy transfer in single photosynthetic complexes.
语种: 英语
内容类型: 期刊论文
URI标识: http://ir.iccas.ac.cn/handle/121111/35723
Appears in Collections:分子动态与稳态结构实验室_期刊论文

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作者单位: 1.Chinese Acad Sci, Inst Chem, State Key Lab Struct Chem Unstable & Stable Speci, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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