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ICCAS OpenIR  > 分子纳米结构与纳米技术实验室  > 期刊论文
题名: Post-annealing of MAPbI(3) perovskite films with methylamine for efficient perovskite solar cells
作者: Jiang, Yan1; Juarez-Perez, Emilio J.1; Ge, Qianqing2; Wang, Shenghao1; Leyden, Matthew R.1; Ono, Luis K.1; Raga, Sonia R.1; Hu, Jinsong2; Qi, Yabing1
刊名: MATERIALS HORIZONS
发表日期: 2016-11-01
卷: 3, 期:6, 页:548-555
收录类别: SCI
英文摘要: An organo-metal halide perovskite is a promising material for solar cell applications, but the polycrystalline nature of perovskites can cause thin films to be non-uniform with disconnected grains. These grain boundaries make the perovskite film vulnerable to the local chemical environment, or allow unwanted direct contact of the electron transporting layer and the hole transporting layer, increasing carrier recombination. We show that post-annealing with methylamine greatly reduces impurities at perovskite grain boundaries and promotes continuity between adjacent grains. When methylamine post-annealed perovskite films are compared to thermally or solvent-annealed films, the carrier lifetime is increased by 3 times. The recombination resistance for the planar perovskite solar cells with the methylamine post-annealing treatment is increased more than 10 times, and the efficiency is increased by 43.1% and 20.0% with respect to the thermally annealed and solvent-annealed perovskite solar cells, respectively. In addition, we show that methylamine post-annealed, meso-structured perovskite solar cells exhibited a power conversion efficiency of up to 18.4%, with significantly improved stability.
语种: 英语
内容类型: 期刊论文
URI标识: http://ir.iccas.ac.cn/handle/121111/35501
Appears in Collections:分子纳米结构与纳米技术实验室_期刊论文

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作者单位: 1.Okinawa Inst Sci & Technol Grad Univ OIST, Energy Mat & Surface Sci Unit EMSS, 1919-1 Tancha Onna Son, Onna, Okinawa 9040495, Japan
2.Chinese Acad Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Inst Chem, Beijing 100190, Peoples R China
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